Most easiest would be the “newer” countries such as most post independence African countries, ex Soviet and Yugoslav nations, with a few island nations thrown in.
The hardest would be ancients and medieval coinage due to age, forgeries and the rarity of gold and silver coins, which would also apply for most other nations if they existed when precious metal coinage was struck for circulation.
Even if you excluded precious metal coins you’ll still need to be patient and have a deep wallet to even make a dent in some countries.
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